Movie S1.

Direct observation of the reactive interface, shown in Fig. 3C. Each frame is the average of 10 images. Movie is a montage of approx. 25 min and runs at 5 fps. Contrast scale: −0.33 to +0.32. (Unless noted otherwise, scale bars in Movies S1–S5: 1 µm.) Movies S1–S5 frame rates are given in femtopicoseconds and compared with the real-time rate in hertz.

Visualization of the spontaneous emergence of a complex, dynamic, and autocatalytic system

Jaime Ortega-Arroyo, Andrew J. Bissette, Philipp Kukura, and Stephen P. Fletcher

PNAS. 2016. 113:11122-11126 DOI: 10.1073/pnas.1602363113